Attaining record-high magnetic exchange, magnetic anisotropy and blocking barriers in dilanthanofullerenes
Abstract
While the blocking barrier (Ueff) and blocking temperature (TB) for "Dysprocenium" SIMs have been increased beyond liquid N2 temperature, device fabrication of these molecules remains a challenge as low-coordinate Ln3+ complexes are very unstable. Encapsulating the lanthanide ion inside a cage such as a fullerene (called endohedral metallofullerene or EMF) opens up a new avenue leading to several Ln@EMF SMMs. The ab initio CASSCF calculations...
Paper Details
Title
Attaining record-high magnetic exchange, magnetic anisotropy and blocking barriers in dilanthanofullerenes
Published Date
Jan 1, 2021
Journal
Volume
12
Issue
42
Pages
14207 - 14216
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