Original paper
Experimental Tests of a Theoretically Predicted Noncausal Correlation between Dynamics and Thermodynamics in Glass-forming Polymer Melts
Abstract
The connection between slow activated relaxation in glass-forming liquids and various equilibrium thermodynamic properties remains intensely debated. The microscopic elastically collective nonlinear Langevin equation theory, a force-level approach that causally relates the structure and dynamics, describes the activated relaxation as a mixed local–nonlocal process involving local caging constraints coupled with longer-range collective...
Paper Details
Title
Experimental Tests of a Theoretically Predicted Noncausal Correlation between Dynamics and Thermodynamics in Glass-forming Polymer Melts
Published Date
Oct 21, 2021
Journal
Volume
54
Issue
21
Pages
10086 - 10099
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Notes
History