Design of 2D Layered Catalyst by Coherent Heteroepitaxial Conversion for Robust Hydrogen Generation

The structural engineering of 2D layered materials is emerging as a powerful strategy to design catalysts for high‐performance hydrogen evolution reaction (HER). However, the ultimate test of this technology under typical operating settings lies in the reduced performance and the shortened lifespan of these catalysts. Here, a novel approach is proposed to design efficient and robust HER catalysts through out‐of‐plane deformation of 2D...