Extremely Tough, Puncture-Resistant, Transparent, and Photoluminescent Polyurethane Elastomers for Crack Self-Diagnose and Healing Tracking

Ensuring material performance reliability and lifetime is crucial for practical operations. Small cracks on the material surface are often detrimental to its safe operation. This study describes the development of a hydrogen bond-rich puncture-resistant polyurethane elastomer with supertoughness. The as-prepared polyurethane transparent films feature high tensile break strength (57.4 MPa) and great toughness (228 MJ m-3). Additionally, a facile,...