Quantum mechanics

Materials science

Nanophotonics

Physical chemistry

Polarization (electrochemistry)

Laser

Physics

Nonlinear system

Dipole

Optics

Nonlinear optics

Resonator

Chemistry

Second-harmonic generation

Optoelectronics

Advanced Science

Dynamical tuning of the nonlinear optical wavefront allows for a specific spectral response of predefined profiles, enabling various applications of nonlinear nanophotonics. This study experimentally demonstrates the dynamical switching of images generated by an ultrathin silicon nonlinear metasurface supporting a high-quality leaky mode, which is formed by partially breaking a bound-state-in-the-continuum (BIC) generated by the collective magnetic dipole (MD) resonance excited in the subdiffractive periodic systems. Such a quasi-BIC MD state can be excited directly under normal plane wave incidence and leads to a strong near-field enhancement to further boost the nonlinear process, resulting in a 500-fold enhancement of the third-harmonic emission experimentally. Due to sharp spectral features and asymmetry of the unit cell, it allows for effective tailoring of the nonlinear emissions over spectral or polarization responses. Dynamical nonlinear image tuning is experimentally demonstarted via polarization and wavelength control. The results pave the way for nanophotonics applications such as tunable displays, nonlinear holograms, tunable nanolaser, and ultrathin nonlinear nanodevices with various functionalities.

Dynamic Nonlinear Image Tuning through Magnetic Dipole Quasi‐BIC Ultrathin Resonators