High harmonic generation

Materials science

Chromatography

Cascade

Extreme ultraviolet

Telecommunications

Computer science

Laser

Physics

Optics

Pulse shaping

Pulse compression

Chemistry

Radar

Femtosecond

Optoelectronics

Attosecond

Carrier-envelope phase

Ultrashort pulse

Science Advances

The advancement of contemporary ultrafast science requires reliable sources to provide high-energy few-cycle light pulses. Through experiments and simulations, we demonstrate an arrangement of pulse postcompression, referred to as cascaded focus and compression (CASCADE), for generating millijoule-level, single-cycle pulses in a compact fashion. CASCADE is realized by a series of foci in matter, whereas pulse compression is provided immediately after each focus to maintain a high efficiency of spectral broadening. By implementing four stages of CASCADE in argon cells, we achieve 50-fold compression of millijoule-level pulses at 1030 nanometers from 157 to 3.1 femtoseconds, with an output pulse energy of 0.98 millijoules and a transmission efficiency of 73%. When driving high harmonic generation, these single-cycle pulses enable the creation of a carrier-envelope phase-dependent extreme ultraviolet continuum with energies extending up to 180 electron volts, providing isolated attosecond pulses at the output.

Nonlinear compression toward high-energy single-cycle pulses by cascaded focus and compression