Atomistic structural mechanism for the glass transition: Entropic contribution
Abstract
A popular Adam--Gibbs scenario has suggested that the excess entropy of glass and liquid over crystal dominates the dynamical arrest at the glass transition with exclusive contribution from configurational entropy over vibrational entropy. However, an intuitive structural rationale for the emergence of frozen dynamics in relation to entropy is still lacking. Here we study these issues by atomistically simulating the vibrational, configurational,...
Paper Details
Title
Atomistic structural mechanism for the glass transition: Entropic contribution
Published Date
Jan 28, 2020
Journal
Volume
101
Issue
1
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