Highly Selective CO2 Capture and Its Direct Photochemical Conversion on Ordered 2D/1D Heterojunctions

Polymeric carbon nitrides (CNs) are regarded as the most sustainable materials for solar energy conversion via photocatalytic processes. However, the first-generation CNs suffered from imperfect charge separation and insufficient CO2 adsorption. Herein, the construction of a heterojunction material involving highly crystalline CN-nanorods with ordered alignment on graphene is delineated, which improves light harvesting, CO2 capture, and...