Time-dependent simulation of photocurrent-detected two-dimensional spectroscopy of open systems.
Abstract
A new time-domain simulation protocol of two-dimensional electronic spectra with photocurrent detection is presented. Time-dependent density functional theory for open systems at finite temperature is applied to evaluate the photocurrent response to four laser pulses, and a non-perturbative phase-matching approach is implemented to extract the fourth-order photocurrent signal with a desired phase-matching condition. Simulations for an open...
Paper Details
Title
Time-dependent simulation of photocurrent-detected two-dimensional spectroscopy of open systems.
Published Date
Nov 18, 2021
Journal
Volume
155
Issue
19
Pages
194113
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