Highly Porous Poly(arylene cyano-vinylene) Beads Derived through the Knoevenagel Condensation of the Oil-in-Oil-in-Oil Double Emulsion Templates

Published on Oct 19, 2021in ACS Macro Letters6.903
· DOI :10.1021/ACSMACROLETT.1C00457
Tomaž Kotnik1
Estimated H-index: 1
,
Gregor Žerjav10
Estimated H-index: 10
+ 2 AuthorsSebastijan Kovačič20
Estimated H-index: 20
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Abstract
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References38
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Photocatalysis with stable, efficient and inexpensive metal-free catalysts is one of the most promising options for non-polluting energy production. This review article covers the state-of-the-art development of various effective metal-free polymeric photocatalysts with large π-conjugated units for chemical transformations including water splitting, CO2 and N2 reduction, organic synthesis and monomer polymerisation. The article starts with the catalytic mechanisms of metal-free photocatalysts. T...
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Abstract A simple structural design principle of poly(arylene ethynylene) π-conjugated microcellular polymers as the pure organic, heterogeneous photocatalytic systems is presented. They are synthesized by the Sonogashira cross-coupling polymerization of 1,3,5-triethynylbenzene and 1,4-diiodobenzene, 2,5-dimethoxy-1,4-diiodobenzene or 2,6-diiodo-4-nitrophenol within the high internal phase emulsion (HIPE). Such poly(arylene ethynylene)-based polyHIPEs allow for fine alignment of the valence and ...
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The formation of carbon–carbon bonds is a quest that has required a lot of research throughout the last 125 years of history of chemistry. The creation of these bonds is key to producing a wide var...
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Emulsions are mixtures of two immiscible liquids in which droplets of one are dispersed in a continuous phase of the other. The most common emulsions are oil–water systems, which have found widespr...
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Conjugated porous polymers (CPPs) are a class of amorphous polymer networks that are, in their design, fully cross-linked and fully π-conjugated. The cross-linked nature of CPPs means that they have permanent intrinsic porosity (on the nanometer scale), which, in combination with the fully π-conjugated framework, makes these materials unique among the wider class of porous polymeric materials. In recent years, the need for new and efficient functional materials has driven the development of CPPs...
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Vinylene-bridged covalent organic frameworks (COFs) have shown great potential for advanced applications due to their high chemical stability and intriguing semiconducting properties. Exploring new...
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