Fundamental Aspects of Enhancing Low-Temperature CO2 Splitting to CO on a Double La2NiFeO6 Perovskite
Abstract
This paper addresses the synergistic effect of binary Ni–Fe sites in double La2NiFeO6 perovskite on low-temperature CO2 conversion to CO in the reverse water–gas shift-chemical looping process. Experimental investigations and DFT calculations proved that, for the reduction of perovskite, the Ni-site facilitates the formation of surface oxygen vacancies and the adsorption of hydrogen with agile lattice oxygen mobility. Thus, incorporating Ni can...
Paper Details
Title
Fundamental Aspects of Enhancing Low-Temperature CO2 Splitting to CO on a Double La2NiFeO6 Perovskite
Published Date
Sep 17, 2021
Journal
Volume
11
Issue
19
Pages
12220 - 12231
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