Theory of the effect of external stress on the activated dynamics and transport of dilute penetrants in supercooled liquids and glasses
Abstract
We generalize the self-consistent cooperative hopping theory for a dilute spherical penetrant or tracer activated dynamics in dense metastable hard sphere fluids and glasses to address the effect of external stress, the consequences of which are systematically established as a function of matrix packing fraction and penetrant-to-matrix size ratio. All relaxation processes speed up under stress, but the difference between the penetrant and matrix...
Paper Details
Title
Theory of the effect of external stress on the activated dynamics and transport of dilute penetrants in supercooled liquids and glasses
Published Date
Aug 4, 2021
Volume
155
Issue
5
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