Femtosecond pulse shaping

Pulse shaping

Optics

Physics

Chirp

Frequency comb

Interferometry

Femtosecond

Ultrashort pulse

Chemistry

Quantum cascade laser

Cascade

Chromatography

Laser

Picosecond

Mode-locking

Nature Photonics

The quantum cascade laser has evolved to be a compact, powerful source of coherent mid-infrared light; however, its fast gain dynamics strongly restricts the formation of ultrashort pulses. As such, the shortest pulses reported so far were limited to a few picoseconds with some hundreds of milliwatts of peak power, strongly narrowing their applicability for time-resolved and nonlinear experiments. Here we demonstrate an approach capable of producing near-transform-limited subpicosecond pulses with several watts of peak power. Starting from a frequency-modulated phase-locked state, ultrashort high-peak-power pulses are generated via spectral filtering, gain modulation-induced spectral broadening and external pulse compression. We assess their temporal nature by means of a novel asynchronous sampling method, coherent beat note interferometry and interferometric autocorrelation. These results open new pathways for nonlinear physics in the mid-infrared.

Femtosecond pulses from a mid-infrared quantum cascade laser