Controlling anisotropic dipolar interaction with shielding resonance in a three-dimensional molecular quantum gas

Published on Mar 10, 2021in arXiv: Quantum Gases
Jun-Ru Li7
Estimated H-index: 7
William G. Tobias3
Estimated H-index: 3
+ 8 AuthorsJun Ye126
Estimated H-index: 126
Ultracold polar molecules possess long-range, anisotropic, and tunable dipolar interactions, providing unique opportunities to probe novel quantum phenomena. However, experimental progress has been hindered by excessive two-body loss, which also limits further cooling via evaporation. Recent work shows the loss can be mitigated by confining molecules in a two-dimensional geometry. However, a general approach for tuning molecular interactions in a full three-dimensional (3D) stable system has been lacking. Here, we demonstrate the use of an electric field-induced shielding resonance to suppress the reactive loss by a factor of 30 while preserving elastic, long-range dipolar interactions in a bulk gas of ultracold 40K87Rb molecules in 3D. The favorable ratio of elastic to inelastic collisions enables direct thermalization, the rate of which depends on the angle between the collisional axis and the dipole orientation controlled by an external electric field. This is a direct manifestation of the anisotropic dipolar interaction. We further achieve dipolar-interaction-mediated evaporative cooling in 3D. This work demonstrates control of a long-lived bulk quantum gas system with tunable long-range interactions, paving the way for the study of collective quantum many-body physics.
Cited By2
#1Yu Liu (CU: University of Colorado Boulder)H-Index: 1
#2Kang-Kuen Ni (Harvard University)H-Index: 25
Advances in atomic, molecular, and optical (AMO) physics techniques allowed the cooling of simple molecules down to the ultracold regime (\lesssim1 mK), and opened the opportunities to study chemical reactions with unprecedented levels of control. This review covers recent developments in studying bimolecular chemistry at ultralow temperatures. We begin with a brief overview of methods for producing, manipulating, and detecting ultracold molecules. We then survey experimental works that explo...
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