Kinetics of NH3 oxidation on Pt/Al2O3: Rate enhancement and NH3 inhibition
Abstract
We describe a combined experimental kinetics and modeling study for NH3 oxidation on Pt/Al2O3 and development of a predictive microkinetic model valid over a range of conditions. The NH3 oxidation rate (TOF) dependence is reported for NH3 concentrations between 10 and 25,000 ppm and temperatures below 250°C for Pt/Al2O3 powder and washcoated monoliths. The data reveal a shift from positive- to negative-order rate dependence on NH3 with the rate...
Paper Details
Title
Kinetics of NH3 oxidation on Pt/Al2O3: Rate enhancement and NH3 inhibition
Published Date
Aug 1, 2021
Journal
Volume
417
Pages
128273 - 128273
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