Enantioselective C(sp3)–H Amidation of Thioamides Catalyzed by a CobaltIII/Chiral Carboxylic Acid Hybrid System
Abstract
Recent advances in Cp x M III catalysis (M=Co, Rh, Ir) have enabled a variety of enantioselective C(sp 2 )−H functionalization reactions, but enantioselective C(sp 3 )−H functionalization is still largely unexplored. We describe an asymmetric C(sp 3 )−H amidation of thioamides using an achiral Co III /chiral carboxylic acid hybrid catalytic system, which provides easy and straightforward access to chiral β‐amino thiocarbonyl and β‐amino carbonyl...
Paper Details
Title
Enantioselective C(sp3)–H Amidation of Thioamides Catalyzed by a CobaltIII/Chiral Carboxylic Acid Hybrid System
Published Date
Dec 20, 2018
Journal
Volume
131
Issue
4
Pages
1165 - 1169
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