Charge transfer kinetics at the solid–solid interface in porous electrodes
Abstract
Interfacial charge transfer is widely assumed to obey the Butler-Volmer kinetics. For certain liquid-solid interfaces, the Marcus-Hush-Chidsey theory is more accurate and predictive, but it has not been applied to porous electrodes. Here we report a simple method to extract the charge transfer rates in carbon-coated LiFePO4 porous electrodes from chronoamperometry experiments, obtaining curved Tafel plots that contradict the Butler-Volmer...
Paper Details
Title
Charge transfer kinetics at the solid–solid interface in porous electrodes
Published Date
Apr 3, 2014
Journal
Volume
5
Issue
1
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